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16届亚运会期间广州城区PM2.5化学组分特征及其对霾天气的影响
摘要点击 4618  全文点击 1677  投稿时间:2012-04-19  修订日期:2012-06-20
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中文关键词  亚运会  PM2.5  化学组分    大气消光系数
英文关键词  Asian Games  PM2.5 aerosol  chemical composition  haze  light extinction coefficient
作者单位E-mail
陶俊 环境保护部华南环境科学研究所,广州 510655 taojun@scies.org 
柴发合 中国环境科学研究院,北京 100012 chaifh@craes.org.cn 
高健 中国环境科学研究院,北京 100012  
曹军骥 中国科学院地球环境研究所,西安 710075  
刘随心 中国科学院地球环境研究所,西安 710075  
张仁健 中国科学院大气物理研究所,北京 100029  
中文摘要
      于2010年11月4~30日在广州城区每天昼夜各采集一个PM2.5样品.对样品进行有机碳、元素碳和水溶性离子分析,同步收集了在线PM2.5浓度、大气消光系数(bext)以及气象因子,探讨了PM2.5特征及其与大气消光系数的关系,并利用修正后的IMPROVE消光系数方程重建大气消光系数.结果发现:亚运期间PM2.5日均值质量浓度为(77.0±24.4)μg·m-3,比亚运前低27.8%. PM2.5和相对湿度是导致霾天气的重要因素. 亚运期间大气消光系数为418 Mm-1,比亚运前低28.3%,(NH4)2SO4、POM (particulate organic material)和LAC(light-absorbing carbon)是主要贡献因子,贡献率达到87.0%.广州及其周边城市采取的减排措施对于缓解亚运期间广州城区的霾天气作用明显.
英文摘要
      Aerosol samples for PM2.5 were collected days and nights from 4 to 30 November 2010 in Guangzhou. The concentrations of organic carbon, element carbon, and water-solubility ions of all particle samples were determined by thermal/optical carbon analyzer and ion chromatography, respectively. In-situ online PM2.5 mass concentrations, light extinction coefficients (bext), and selected meteorological parameters for this period were also measured. Temporal variation of PM2.5 mass concentrations and its relationship with bext were discussed, and bext was reconstructed by revised IMPROVE formula. The results showed that the average mass concentration of PM2.5 was (77.0±24.4) μg·m-3 during the Asian Games period, which was 27.8% lower than that of the period before Asian Games. PM2.5 and relative humidity were the dominant factors contributing to hazy weather. The average value of bext was 418 Mm-1 during the Asian Games period, which was 28.3% lower than that of the period before Asian Games. The major contributors to bext included (NH4)2SO4, POM, and LAC, which accounted for 87.0% of bext during the Asian Games period. A series of stringent air quality control measures were implemented by the Guangzhou Municipal Government and other cooperative cities, which greatly alleviated the hazy weathers in Guangzhou urban area during the Asian Games period.

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