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调水调沙对黄河下游颗粒有机碳输运的影响
摘要点击 1518  全文点击 1106  投稿时间:2015-01-11  修订日期:2015-03-21
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中文关键词  黄河  调水调沙  颗粒有机碳  稳定碳同位素  输运
英文关键词  Yellow River  water and sediment regulation  particulate organic carbon  stable carbon isotope  transport
作者单位E-mail
张婷婷 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
zhtt_2012@163.com 
姚鹏 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
海洋科学与技术青岛协同创新中心, 青岛 266100
中国海洋大学海洋有机地球化学研究所, 青岛 266100 
yaopeng@ouc.edu.cn 
王金鹏 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
 
潘慧慧 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
 
高立蒙 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
 
赵彬 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
 
李栋 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
中国海洋大学化学化工学院, 青岛 266100 
 
中文摘要
      流域内各种自然过程及人为活动对河流有机碳的输运都会产生影响,而正确认识河流有机碳的输运过程是全球碳循环研究的重要方面. 于2012年调水调沙期间(6月19日至7月20日)在黄河利津采集了表层悬浮颗粒物,进行了粒度组成、颗粒有机碳(particulate organic carbon,POC)及其稳定同位素丰度(δ13C)等参数的分析,用来研究调水调沙期间POC的来源、组成和丰度的变化规律与影响因素. 结果表明,2012年黄河调水调沙可以根据径流量和输沙量的变化分为排水和排沙两个阶段,这两个阶段黄河水沙及POC和δ13C的变化,体现了调水调沙对颗粒物及其赋存有机碳来源的影响. 排水阶段径流量高达4270 m3·s-1,下游河道被冲刷,使底层泥沙再悬浮,因此这一阶段颗粒物粒径较粗(平均中值粒径13.9 μm),有机碳含量较低(平均0.38%),δ13C偏正且稳定(-24.2‰ ± 0.3‰),可能与底层泥沙中POC年龄较老、降解程度高有关; 排沙阶段含沙量大(可达17.8 kg·m-3),颗粒物较细(平均中值粒径5.9 μm),有机碳含量较高(平均0.50%),δ13C偏负且波动较大(-24.8‰ ± 0.6‰),这与颗粒物主要来自上游水库和下游暴雨冲刷河岸,POC相对新鲜有关. 2012年调水调沙期间POC日通量与输沙量的变化一致,总输送量约为1.13×105 t,占全年POC输送量的12%. 与往年相比,2012年黄河调水调沙时期径流量增大,但输沙量和POC通量有所减小. 由此可见,调水调沙对黄河颗粒有机碳的输运有重要影响,而颗粒有机碳在调水调沙期间不同阶段也有明显不同的来源、组成和输运模式.
英文摘要
      Both natural processes and human activities in river basins have important impacts on the transport of riverine organic carbon (OC). Better understanding of the riverine OC transport processes is critical for the studies of global carbon cycling. Suspended particulate matters collected from the Lijin Station in the lower Yellow River during the water and sediment regulation (WSR) period in 2012 (19 June-20 July) were analyzed for grain size, particulate OC (POC) and stable carbon isotopic ratios (δ13C) to investigate the sources, composition, abundance of POC and the effect of WSR on the transport of POC. The results showed that the WSR in 2012 could be divided into two stages according to the variation of water and sediment discharges: the water-release stage (WRS) and the sediment-release stage (SRS). Variations of the water discharge, sediments, POC and δ13C in these two stages reflected the impacts of WSR on the sources of particulate matters and associated OC. The water discharge in the WRS stage was the highest (4270 m3·s-1), and the sediments scoured from the riverbed in the lower reaches were the major source of suspended particulate matters in this stage, therefore the particles were characterized by relatively coarse grain size (13.9 μm in average of median grain size), low POC (avg. 0.38%) and relatively enriched and constant δ13C (-24.2‰±0.3‰), probably because POC in the sediments scoured from the riverbed had old radiocarbon ages and high degradation. The suspended particulate matters in the SRS stage were mainly derived from the upstream reservoirs and flushed riverbanks due to local rainstorm, and the POC age was relatively young, thus this stage was characterized by high concentration of suspended particulate matters (up to 17.8 kg·m-3), fine particles (5.9 μm in average of median grain size), high POC (avg. 0.50%), and depleted and varied δ13C values (-24.8‰±0.6‰). Variation of daily POC flux had similar pattern with sediment discharge, and the total POC flux during the water and sediment regulation period was 1.13×105 tons, accounting for 12% of the total POC flux in 2012. Compared with previous years, the total water discharge during the WSR period in 2012 has increased, while the total sediment flux and POC flux have reduced. In general, WSR played an important role on the transport of POC in the Yellow River. And furthermore, there was significant difference in the sources, composition and transport of POC in different stages of WSR.

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