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冬季猪粪固体堆放过程中NH3、N2O和NO排放特征研究
摘要点击 1586  全文点击 1198  投稿时间:2013-10-25  修订日期:2014-01-09
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中文关键词  NH3  N2O  NO  温室气体  固体堆放  翻堆
英文关键词  NH3  N2O  NO  greenhouse gas  manure storage  pile-turning
作者单位E-mail
丁钢强 广东工业大学环境科学与工程学院, 广州 510006
中国科学院大气物理研究所, 北京 100029 
gangqiangd@126.com 
韩圣慧 中国科学院大气物理研究所, 北京 100029 shenghui_han@post.iap.ac.cn 
袁玉玲 湖南农业大学资源环境学院, 长沙 410128  
罗琳 湖南农业大学资源环境学院, 长沙 410128  
王立刚 中国农业科学院农业资源与农业区划研究所, 北京 100081  
李虎 中国农业科学院农业资源与农业区划研究所, 北京 100081  
李萍 广东工业大学环境科学与工程学院, 广州 510006  
中文摘要
      针对农村猪粪典型处理方式中的固体堆放管理,研究猪粪在冬季(2012年11月~2013年2月)固体堆放过程中NH3、N2O和NO排放特征. 实验共设两个处理——无覆盖(non-covered,NC)和水稻秸秆覆盖(covered,C),堆放时间为73 d,期间进行了3次翻堆操作. 实验观测了3种含氮气体(NH3、N2O和NO)的排放通量和堆体剖面N2O浓度变化. 结果表明,猪粪固体堆放过程中NH3、N2O和NO排放累积量(以N计)分别占初始TN的比例为2.1%~2.6%、0.02%和~0.00025%. 两个处理的含氮气体排放通量变化趋势基本一致,且有覆盖堆体的含氮气体的排放量略低于无覆盖堆体. 在堆放初期,NH3排放量最先出现峰值,之后N2O和NO排放开始增加. NH3和NO在固体堆放的中前期呈现互为消长的变化趋势; 到堆放后期,N2O开始出现比前期高出两倍的排放高峰,而NH3和NO出现小幅增长. 翻堆前后,NH3的排放无明显变化,而N2O排放在翻堆后均出现降低的变化,NO排放却出现升高的变化.
英文摘要
      Swine manure solid storage is a typical management in rural area of China. In order to investigate the characteristics of NH3, N2O and NO emissions during manure storage in winter (Nov., 2012 to Feb., 2013), two treatments were conducted: non-covered (NC) and covered (C) with straws, and each treatment had three times of pile-turning during the 73 days storage. The emission fluxes of three nitrogen gases (NH3, N2O and NO) were measured and the profile-N2O concentrations inside the swine pile profile and in the soil under the pile were also measured. The results indicated that 2.1%-2.6%, 0.02% and ~0.00025% of total nitrogen were lost in the form of NH3, N2O and NO respectively during the whole swine manure solid storage. The nitrogen gases in the two treatments had the same variation characteristics, but all the nitrogen gases were reduced in the covered treatment. In the early storage stage, NH3 emission peak occurred first and then the emissions of N2O and NO started increasing. In the middle storage stage, the emissions of NH3 and NO showed mutual growth and decline trend. In the late storage stage, N2O emission peak was twice higher than that in the early stage, while NH3 and NO emissions showed a slight increase. Before and after pile-turning operation, NH3 emission had little change, but N2O emission was decreasing and NO emission was rising after pile-turning.

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