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深圳市2022年春季新冠疫情管控期间空气质量分析
摘要点击 1788  全文点击 1018  投稿时间:2022-05-29  修订日期:2022-09-02
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中文关键词  疫情管控  华南  春季  臭氧污染  协同控制
英文关键词  COVID-19 lockdown  SouthChina  spring  ozone pollution  collaborative control
作者单位E-mail
刘婵芳 广东省深圳生态环境监测中心站, 深圳 518049 99753846@qq.com 
张傲星 南方科技大学环境科学与工程学院, 深圳 518055 zhangax@sustech.edu.cn 
房庆 广东省深圳生态环境监测中心站, 深圳 518049  
叶毓婧 广东省深圳生态环境监测中心站, 深圳 518049  
杨红龙 深圳市国家气候观象台, 深圳 518040  
陈炯恺 南方科技大学环境科学与工程学院, 深圳 518055  
吴雯潞 南方科技大学环境科学与工程学院, 深圳 518055  
侯岳 南方科技大学环境科学与工程学院, 深圳 518055  
莫佳佳 南方科技大学环境科学与工程学院, 深圳 518055  
傅宗玫 南方科技大学环境科学与工程学院, 深圳 518055  
中文摘要
      短期减排是我国城市应对大气污染事件的重要应急管控手段,但短期减排的效益尚未得到完善分析.2022年3月14~20日,广东省深圳市为抑制新冠疫情传播实施了全市管控,为评估短期减排对华南城市春季空气质量的影响提供独特机会.结合深圳市高精度环境空气质量监测与气象观测等多源数据,分析了深圳市管控期间前后的空气质量变化.此次管控前和管控期中均有部分日期天气形势静稳,局地污染水平主要反映本地排放,有利于分析本地减排的影响.观测与WRF-GC区域化学模拟都表明,与珠三角周边城市相比,深圳市管控期间由于市内交通源排放显著减少,深圳市二氧化氮(NO2)浓度降低(-26±9.5)%,可吸入颗粒物(PM10)浓度降低(-28±6.4)%,细颗粒物(PM2.5)浓度降低(-20±8.2)%,但臭氧(O3)浓度无显著变化[(-1.0±6.5)%].TROPOMI卫星观测的甲醛和二氧化氮柱浓度数据对比表明,2022年春季珠三角臭氧光化学主要受挥发性有机物(VOCs)浓度控制,对氮氧化物浓度降低不敏感,反而可能因氮氧化物对臭氧滴定效应减弱而造成臭氧浓度上升.由于较小的减排时空范围,该城市尺度短期减排造成的空气质量效应略弱于我国各地在2020年大范围疫情管控期间的空气质量影响.华南城市未来空气质量治理,应当关注氮氧化物削减对臭氧污染的影响,并更多地考虑氮氧化物与VOCs的协同减排方案.
英文摘要
      The short-term reduction of air pollutant emissions is an important emergency control measure for avoiding air pollution exceedances in Chinese cities. However, the impacts of short-term emission reductions on the air qualities in southern Chinese cities in spring has not been fully explored. We analyzed the changes in air quality in Shenzhen, Guangdong before, during, and after a city-wide lockdown associated with COVID-19 control during March 14 to 20, 2022. Stable weather conditions prevailed before and during the lockdown, such that local air pollution was strongly affected by local emissions. In-situ measurements and WRF-GC simulations over the Pearl River Delta (PRD) both showed that, due to reductions in traffic emissions during the lockdown, the concentrations of nitrogen dioxide (NO2), respirable particulate matter (PM10), and fine particulate matters (PM2.5) in Shenzhen decreased by (-26±9.5)%, (-28±6.4)%, and (-20±8.2)%, respectively. However, surface ozone (O3) concentration did not change significantly[(-1.0±6.5)%]. TROPOMI satellite observations of formaldehyde and nitrogen dioxide column concentrations indicated that the ozone photochemistry in the PRD in spring 2022 was mainly controlled by the volatile organic compound (VOCs) concentrations and was not sensitive to the reduction in nitrogen oxide (NOx) concentrations. Reduction in NOx may even have increased O3, because the titration of O3 by NOx was weakened. Due to the small spatial-temporal extent of emission reductions, the air quality effects caused by this short-term urban-scale lockdown were weaker than the air quality effects across China during the widespread COVID-19 lockdown in 2020. Future air quality management in South China cities should consider the impacts of NOx emission reduction on ozone and focus on the co-reduction scenarios of NOx and VOCs.

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