| 福建茫荡山地区春季大气O3、HONO、HCHO、H2O2对 ·OH的贡献率研究 |
| 摘要点击 3211 全文点击 1819 投稿时间：2012-12-24 修订日期：2013-03-20 |
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| 中文关键词 ·OH 山区观测 O3 HONO HCHO H2O2 |
| 英文关键词 ·OH mountain observation O3 HONO HCHO H2O2 |
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| 中文摘要 |
| 2009年春季在福建南平市茫荡山地区进行观测,测量了 ·OH源O3、HONO、HCHO和H2O2的浓度. 结果表明O3、HCHO、HONO、H2O2浓度分别为4.96×10-8、3.97×10-10、2.53×10-10、1.18×10-10,低于华北农村的浓度. 利用CMAQ计算O3、HCHO、HONO、H2O2对 ·OH的贡献率,分别为57.0%、7.7%、34.9%、0.4%. O3光解是该地区最重要的 ·OH来源. O3、HCHO、H2O2对 ·OH的贡献呈现单峰变化,在12:00~13:00达到峰值. HONO对 ·OH的贡献曲线呈波动状,和人类居住环境清晨出现峰值的情况不同. |
| 英文摘要 |
| The observation was conducted in Mangdang Mountain, Nanping, Fujian Province in the spring of 2009. Ozone, HONO, HCHO and H2O2 which are regarded as the sources of ·OH and other atmospheric components were measured. Mixing ratios of O3, HCHO, HONO and H2O2 were determined to be 4.96×10-8, 3.97×10-10, 2.53×10-10 and 1.18×10-10 respectively, which were lower than the previous observation at the rural areas in Northern China. Using CMAQ, the contribution factors to the ·OH of O3, HCHO, HONO, and H2O2 were calculated to be 57.0%, 7.7%, 34.9% and 0.4% respectively. The photolysis of O3 was the most important source of OH radicals in the atmosphere. The contribution factors of O3, HCHO, and H2O2 had a single peak during 12:00-13:00 local time. For HONO, the contribution factor showed fluctuations during the daytime, unlike the human living environment in which it peaked in the morning. |
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