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C/N和污泥浓度对以pH值调控的亚硝化系统影响
摘要点击 1401  全文点击 470  投稿时间:2018-07-17  修订日期:2018-08-31
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中文关键词  亚硝化  反硝化  pH值  过程控制  碳氮转化
英文关键词  nitrosation  denitrification  pH value  process control  conversion of carbon and nitrogen
作者单位E-mail
张敏 苏州科技大学环境科学与工程学院, 苏州 215009 15289893686@163.com 
韦佳敏 苏州科技大学环境科学与工程学院, 苏州 215009  
黄慧敏 苏州科技大学环境科学与工程学院, 苏州 215009  
姜滢 苏州科技大学环境科学与工程学院, 苏州 215009  
郭萌蕾 苏州科技大学环境科学与工程学院, 苏州 215009  
陈重军 苏州科技大学环境科学与工程学院, 苏州 215009
江苏省水处理技术与材料协同创新中心, 苏州 215009
江苏省环境科学与工程重点实验室, 苏州 215009 
chongjunchen@163.com 
沈耀良 苏州科技大学环境科学与工程学院, 苏州 215009
江苏省水处理技术与材料协同创新中心, 苏州 215009
江苏省环境科学与工程重点实验室, 苏州 215009 
 
中文摘要
      pH是亚硝化系统实现并稳定的重要调控手段,为研究不同C/N(0、1、2、3、4)及污泥浓度(污泥量:配水量为1:6、1:3、1:1)下亚硝化系统的pH变化规律及在不同pH变化下对污染物去除转化过程的影响,以乙酸钠为碳源,采用锥形瓶接种成熟的亚硝化污泥进行了批次试验.结果表明,相同污泥浓度下,C/N越大,pH增量越大,反硝化效率越高;相同C/N下,污泥浓度越大,pH增量越小,反硝化效率越高.反应系统对碳氮的去除转化与pH变化存在较大的相关性,且反硝化与亚硝化反应具有先后顺序.整个系统运行期间,pH上升过程的比COD去除速率是pH下降时的7~16倍,pH下降过程的比氨氧化速率(SAOR)是上升过程的1~20倍,当pH<6.1,系统失去氨氧化能力.本试验过程中,C/N为4时该系统碳氮去除效率较其他工况最佳,3个污泥浓度下分别耗时480、350、300 min完成氨的转化及80%的COD去除.不同工况下,亚硝化反应在系统内的占比维持在50%以上,且NO3--N浓度一直低于5 mg·L-1,表明该系统以亚硝化作用为主导.
英文摘要
      pH is one of the most important means of control for the realization and stability of the nitrosation system. To study the change rule of pH values of the nitrosation system and the influence of pollution removal and transformation at different pH under the conditions of different C/N (0, 1, 2, 3,4) and sludge concentrations (sludge amount:water content was 1:6, 1:3, 1:1), batch tests were conducted with tapered bottles using sodium acetate as the carbon source and inoculated with mature nitrosation sludge. The results showed that the higher the C/N, the higher the pH increment and the denitrification efficiency at the same sludge concentration. At the same C/N, a higher sludge concentration corresponded to a smaller pH increment but a higher denitrification efficiency. The removal and transformation of carbon and nitrogen was highly correlated with pH changes in the reaction system, and the denitrification and nitrosation reactions were in sequence. Throughout the operational period of the system, as pH increased, the specific organic matter removal rate was 7-16 times as much as when pH decreased. However, as pH decreased, the specific ammonia oxidation rate (SAOR) was 1-20 times that of when pH increased. When pH was less than 6.1, the system lost its ability to oxidize ammonia-nitrogen. The highest removal efficiency of carbon and nitrogen in the system was achieved when C/N was 4. Ammonia transformation 80% COD removal at the three sludge concentrations took 480, 350, and 300 min, respectively. Under different conditions, the proportion of nitrosation in the system remained above 50% and the concentration of NO3--N remained below 5 mg·L-1, which indicated that the system was dominated by nitrosation.

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